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Journal Articles

Application of the Y separation method using DGA resin for the measurement of $^{90}$ Sr in human teeth and marine fish bones

Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Terashima, Motoki

KEK Proceedings 2023-2, p.155 - 160, 2023/11

In this presentation, we report the results of the application of the Y-separation method using DGA resin to the determination of $^{90}$ Sr in human teeth and seawater fish bones.

Journal Articles

Study on the uptake of $^{90}$ Sr and $^{137}$ Cs into wild animals after the Fukushima Daiichi Nuclear Power Plant accident using hard tissue as an indicator

Koarai, Kazuma

Hosha Kagaku, (47), p.24 - 27, 2023/03

Ca-based tissues, such as teeth and bones, are called hard tissues. Sr is incorporated into the tooth during calcification. Once incorporated, it remains until the tooth falls out. Therefore, $^{90}$ Sr in teeth recorded $^{90}$ Sr contamination by the 1F accident in the environment during the formation period. The article presents current research findings.

Journal Articles

Rapid analysis of $^{90}$ Sr in cattle bone and tooth samples by inductively coupled plasma mass spectrometry

Koarai, Kazuma; Matsueda, Makoto; Aoki, Jo; Yanagisawa, Kayo*; Terashima, Motoki; Fujiwara, Kenso; Kino, Yasushi*; Oka, Toshitaka; Takahashi, Atsushi*; Suzuki, Toshihiko*; et al.

Journal of Analytical Atomic Spectrometry, 36(8), p.1678 - 1682, 2021/08

https://doi.org/10.1039/D1JA00086A

Times Cited Count：5 Percentile：55.72(Chemistry, Analytical)

Rapid analysis of $^{90}$ Sr in bone and tooth samples of cattle were achieved by an inductively coupled plasma mass spectrometry (ICP-MS) coupled with mass shift and solid phase extraction techniques. Limit of detection (LOD) in the ICP-MS measurement of 0.1 g samples was lower than that of the radioactivity measurement. Analytical time of the ICP-MS method was reduced from 20 days to 11 hours, compared with the radiometric method. Therefore, the ICP-MS method can be rapid and useful procedure of $^{90}$ Sr in small bone and tooth samples derived from terrestrial animals.

Journal Articles

Vertical distribution of $^{90}$ Sr and $^{137}$ Cs in soils near the Fukushima Daiichi Nuclear Power Station

Sasaki, Takayuki*; Matoba, Daisuke*; Dohi, Terumi; Fujiwara, Kenso; Kobayashi, Taishi*; Iijima, Kazuki

Journal of Radioanalytical and Nuclear Chemistry, 326(1), p.303 - 314, 2020/10

https://doi.org/10.1007/s10967-020-07294-3

Times Cited Count：3 Percentile：35.51(Chemistry, Analytical)

Journal Articles

Rapid determination of Sr-90 in environmental matrices by SPE-ICP-MS for emergency monitoring

Fujiwara, Kenso; Yanagisawa, Kayo*; Iijima, Kazuki

Environmental Radiochemical Analysis VI, p.89 - 96, 2019/09

Since Strontium-90 (Sr-90) is one of the high yield and hazardous fission products, accurate and low-level detection of Sr-90 is essential for environmental samples. Especially, in case of nuclear power plant accidents, rapid and precise assessment of Sr-90 for environmental monitoring and health physics is required. In order to evaluate the migration of radionuclides in the environment, not only Sr-90 in water but also those in soil and biological samples should be measured. A new method for rapid quantification of Sr-90 by online solid phase extraction coupled with inductively coupled plasma mass spectrometry (SPE-ICP-MS) has been developed. In this method, it is unavoidable to eliminate the interference by polyatomic ion (e.g., ArCa, Ca $_{2}$ ) induced by isotopes and matrices in fishes and soil. In this study, SPE-ICP-MS method was applied to the measurement of Sr-90 in fishes, and the influence of the Sr isotopes and coexisting ions such as Ca was evaluated.

Journal Articles

Removal of radioactive substances using inorganic compounds entangled by polymer chain grafted onto fiber

Saito, Kyoichi*; Kojima, Takashi*; Asai, Shiho

Bunseki Kagaku, 66(4), p.233 - 242, 2017/04

https://doi.org/10.2116/bunsekikagaku.66.233

Times Cited Count：1 Percentile：3.41(Chemistry, Analytical)

Insoluble cobalt ferrocyanide and sodium titanate specifically capture cesium and strontium ions, respectively, in water contaminated with radionuclides which is found in Fukushima Daiichi NPP. The inorganic compounds used in this study were formed as precipitates in the polymer chain grafted onto a commercially available 6-nylon fiber using radiation-induced graft polymerization. An impregnation structure with the precipitates entangled by the grafted polymer chain through an electrostatic interaction via multipoints was indicated. The resultant insoluble cobalt ferrocyanide- or sodium titanate-impregnated fiber exhibited a higher adsorption rate and adsorption capacity per gram of the inorganic compound for cesium or strontium ions in seawater than conventional granular adsorbents.

Journal Articles

Anthropogenic radionuclides in seawater of the Japan Sea; The Results of recent observations and the temporal change of concentrations

Ito, Toshimichi; Aramaki, Takafumi*; Otosaka, Shigeyoshi; Suzuki, Takashi; Togawa, Orihiko; Kobayashi, Takuya; Kawamura, Hideyuki; Amano, Hikaru; Senju, Tomoharu*; Chaykovskaya, E. L.*; et al.

Journal of Nuclear Science and Technology, 42(1), p.90 - 100, 2005/01

https://doi.org/10.3327/jnst.42.90

Times Cited Count：14 Percentile：67.84(Nuclear Science & Technology)

During 1996-2002, a wide-area research project on anthropogenic radionuclides was done in the Japanese and Russian EEZ of the Japan Sea to investigate their migration. As the results of expeditions in 2001 and 2002, (1) the concentrations and distributions of radionuclides are similar to the results of previous, (2) inventories of these radionuclides indicate accumulation in the Japan Sea seawater compared to the amounts supplied by global fallout, (3) $^{90}$ Sr and $^{137}$ Cs concentrations in intermediate layer show temporal variations, and 4) the variations may reflect the water mass movement in upper part of the Japan Sea.

Journal Articles

Anthropogenic radionuclides in seawater of the Japan Sea; The Results of recent expeditions carried out in the Japanese and Russian EEZ

Ito, Toshimichi; Aramaki, Takafumi*; Otosaka, Shigeyoshi; Suzuki, Takashi; Togawa, Orihiko; Kobayashi, Takuya; Senju, Tomoharu*; Chaykovskaya, E. L.*; Lishavskaya, T. S.*; Karasev, E. V.*; et al.

Proceedings of International Symposium on Radioecology and Environmental Dosimetry, p.396 - 401, 2003/10

no abstracts in English

Journal Articles

Field tests on migration of TRU-nuclide, 3; Migration test of radionuclide in aerated soil layer

Mukai, Masayuki; Tanaka, Tadao; Maeda, Toshikatsu; Ogawa, Hiromichi; Matsumoto, Junko; Munakata, Masahiro; Zhao, Y.*; Guo, Z.*; Ni, S.*; Li, S.*

Nihon Genshiryoku Gakkai Wabun Rombunshi, 2(3), p.342 - 349, 2003/09

https://doi.org/10.3327/taesj2002.2.342

Evaluation of radionuclide migration in geologic media is of great importance in safety assessment for shallow land disposal specially for TRU nuclides because of inadequate data based on field test. As a cooperative research between JAERI and CIRP, a field test of radionuclide migration was conducted under natural condition using Sr-90, Np-237 and Pu-238 to obtain migration data of the radionuclides in actual aerated layer under natural rainfall condition. Values of input parameters to an existing evaluation equation of nuclide migration were determined on the basis of the results of laboratory experiments of batch and column methods and field investigation. Migration distribution of the radionuclides calculated with the determined values showed reasonable agreement with the measured distribution of the field test. This confirmed an applicability of the evaluation equation for radionuclide migration to actual aerated layer under natural condition.

Journal Articles

Monitoring of potential environmental effects of oil exploration in the Sea of Okhotsk and distribution of artificial radionuclides in the Sea of Japan

Tkalin, A. V.*; Lishavskaya, T. S.*; Belan, T. A.*; Karasev, E. V.*; Togawa, Orihiko

Pacific Oceanography, 1(1), p.42 - 52, 2003/08

no abstracts in English

Journal Articles

Depth profiles of long lived radionuclides in Chernobyl soils sampled around 10 years after the accident

Amano, Hikaru; Onuma, Yoshikazu*

Journal of Radioanalytical and Nuclear Chemistry, 255(1), p.217 - 222, 2003/01

https://doi.org/10.1023/A:1022229209171

Times Cited Count：8 Percentile：49.89(Chemistry, Analytical)

no abstracts in English

Journal Articles

Accumulation and potential dissolution of Chernobyl-derived radionuclides in river bottom sediments

Sanada, Yukihisa*; Matsunaga, Takeshi; Yanase, Nobuyuki; Nagao, Seiya; Amano, Hikaru; Takada, Hideshige*; Tkachenko, Y.*

Applied Radiation and Isotopes, 56(5), p.751 - 760, 2002/04

https://doi.org/10.1016/S0969-8043(01)00274-3

Times Cited Count：14 Percentile：65.6(Chemistry, Inorganic & Nuclear)

Areas contaminated with radionuclides from the Chernobyl nuclear accident have been identified in Pripyat River near the Chernobyl Nuclear Power Plant. The bottom sediments contained $^{137}$ Cs (10 $^{5}$ - 10 $^{6}$ Bq/m $^{2}$ ) within 0-30 cm depth, which is comparable to the ground soil of in the vicinity of the nuclear power plant (the Exclusion Zone). The sediments also accumulated $^{90}$ Sr (10 $^{5}$ Bq/m $^{2}$ ), $^{239,240}$ Pu (10 $^{4}$ Bq/m $^{2}$ ), $^{241}$ Am (10 $^{4}$ Bq/m $^{2}$ ) derived from the accident.The comparison of these inventories with those of the released radionuclides at the accident and the experimental analysis using the selective sequential extraction of the radionuclides in the sediments suggest that the potential mobility of $^{137}$ Cs and $^{239,240}$ Pu is low compared with $^{90}$ Sr in the bottom sediment, while the potential dissolution of $^{90}$ Sr from the river bottom sediment should be taken into account with respect to the long-term radiological influence on the aquatic environment.